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Design, synthesis and application of a new type of bifunctional Le-Phos in highly enantioselective gamma-addition reactions of N-centered nucleophiles to allenoates
A novel class of cyclic phosphine derived bifunctional catalysts (Le-Phos) is reported, which can be readily prepared from inexpensive and commercially available starting materials and exhibit good performances in enantioselective gamma-addition reactions of N-centered nucleophiles and allenoates under mild conditions. The salient features of this reaction include high product yields, good enantioselectivity, mild reaction conditions, and broad substrate scope and gram-scale scalability.
Note that a catalyst decreases the activation energy for both the forward and the reverse reactions and hence accelerates both the forward and the reverse reactions.name: Thiazolidin-2-one, you can also check out more blogs about2682-49-7
Reference£º
Quinuclidine – Wikipedia,
Quinuclidine | C7H417N | ChemSpider